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P. J. H. Baily B.Sc.(Econ.), A.C.I.S., M.Inst.P.S.py. is a supplement to the earlier volumes II/4, II/6, and II/14. The slight change in the title reflects current trends in the applications of spectroscopic methods. Together, the four volumes collect all the critically evaluated data published up to 1989/90 on constants of free molecules obtained