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Titlebook: Coherent Multidimensional Spectroscopy; Minhaeng Cho Book 2019 Springer Nature Singapore Pte Ltd. 2019 light-harvesting complex proteins.I

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The Development of Coherent Multidimensional Microspectroscopy, details about molecular structure and dynamics that are available using coherent multidimensional techniques (CMDS). However, incorporating traditional CMDS techniques into imaging modalities requires tackling obstacles including acquisition time, spatial resolution, and detection methods. Thus, th
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Frequency Comb-Based Multidimensional Coherent Spectroscopy,a multidimensional coherent spectrum rapidly and with unprecedented frequency resolution. To demonstrate the improvements in resolution and data acquisition speed we apply this method to Doppler broadened Rb atoms whose energy level splittings are of the order of hundreds of MHz and measure a rephas
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Nonlinear Spectroscopy of Chromophores in Condensed Phases with Multiple Frequency Combs,le and generates phase-matched coherently emitted electromagnetic fields under detection. To maintain the coherence of the involved electromagnetic fields, each single laser pulse is split into multiple pulses that remain in a fixed relative phase within their coherence lengths. However, multi-comb
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https://doi.org/10.1007/978-3-319-02315-1ence between the two chromophores, and the sensitivity of contributions accessing or originating from doubly electronically excited states of the dimer to the possible presence of an exciton shift all provide physical interpretations of individual wave-packet overlaps.
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https://doi.org/10.1007/978-3-319-10948-0r, made this approach impractical beyond three dimensions. Here, we discuss advances in four-dimensional spectroscopy that addresses, and overcomes, these challenges. We demonstrate that resonance may be used to control which pathways contribute to the signal, thereby greatly simplifying the physica
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