书目名称 | Studies of Photoinduced Molecular Dynamics Using a Fast Imaging Sensor |
编辑 | Craig S. Slater |
视频video | http://file.papertrans.cn/881/880956/880956.mp4 |
概述 | Nominated as an outstanding PhD thesis by the University of Oxford, UK.Includes 85 colour illustrations.Offers an excellent introduction to the field.Includes supplementary material: |
丛书名称 | Springer Theses |
图书封面 |  |
描述 | The work presented in this thesis involves a number of sophisticated experiments highlighting novel applications of the Pixel Imaging Mass Spectrometry (PImMS) camera in the field of photoinduced molecular dynamics. This approach represents the union of a new enabling technology (a multiple memory register, CMOS-based pixel detector) with several modern chemical physics approaches and represents a significant leap forward in capabilities. Applications demonstrated include three-dimensional imaging of photofragment Newton spheres, simultaneous electron-ion detection using a single sensor, and ion-ion velocity correlation measurements that open the door to novel covariance imaging experiments. When combined with Coulomb explosion imaging, such an approach is demonstrated to allow the measurement of molecular structure and motion on a femtosecond timescale. This is illustrated through the controlled photoexcitation of torsional motion in biphenyl molecules and the subsequent real-time measurement of the torsional angle.. |
出版日期 | Book 2016 |
关键词 | Coincidence Imaging; Coulomb Explosion; Covariance Imaging; Ion Imaging; PImMS Camera; Photoion-photoion |
版次 | 1 |
doi | https://doi.org/10.1007/978-3-319-24517-1 |
isbn_softcover | 978-3-319-37391-1 |
isbn_ebook | 978-3-319-24517-1Series ISSN 2190-5053 Series E-ISSN 2190-5061 |
issn_series | 2190-5053 |
copyright | Springer International Publishing Switzerland 2016 |