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Titlebook: Electrosorption; Eliezer Gileadi Book 1967 Plenum Press 1967 Atom.Diffusion.Langmuir.Sorption.adsorption.catalysis.catalyst.electrochemist

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书目名称Electrosorption
编辑Eliezer Gileadi
视频video
图书封面Titlebook: Electrosorption;  Eliezer Gileadi Book 1967 Plenum Press 1967 Atom.Diffusion.Langmuir.Sorption.adsorption.catalysis.catalyst.electrochemist
描述The gradual emergence during the last decade of the study of the mechanism of electrode reactions from the dark ages has given stimulus to a consideration of the double layer at metal-solution interfaces, which extends far outside the classical experimental studies of the capacitance of the mercury solution interface made during the 1950‘s by D. C. Grahame at Amherst College, Massachusetts. The central aspect of the study of an electrode reaction is the elucidation of its path and rate-determining step. Two fields are, however, prerequisites for such studies. First, it must be known what species are in the bulk of the solution, for these will seldom be simple ones such as H30~ and this study ("complex ions") has been made with both extent and depth. Second, the occupancy of the surface of the electrocatalyst and the associated field gradients must be known as a function of position in the double layer. Such "maps of the double layer" can be given with reasonable certainty up to concentrations of about 1 N for mercury in contact with solutions of inorganic ions. However, this is-or was until very recently-the extent of the know­ ledge. The problems confronting a fundamental approach
出版日期Book 1967
关键词Atom; Diffusion; Langmuir; Sorption; adsorption; catalysis; catalyst; electrochemistry; electrolyte; fields; f
版次1
doihttps://doi.org/10.1007/978-1-4684-1731-9
isbn_softcover978-1-4684-1733-3
isbn_ebook978-1-4684-1731-9
copyrightPlenum Press 1967
The information of publication is updating

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https://doi.org/10.1007/978-1-4020-5281-1the solvation of electrodes quantitatively. Exceptions are the attempts that have been made to evaluate the contribution of the . potential to the total potential drop at the metal-solution interface, but even here there is still controversy as to magnitude and even sign (cf. Chapter 5 on potentials of zero charge).
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Ye Yaoxian,Niu Zezhen,Huang Jiguanglayer; . is the Faraday; .. is the charge of the ionic species ., including the sign; and .. is the surface excess of that component in the interphase, in moles per unit area of the interface. The charge on the solution side of the double layer .. is equal and opposite in sign to the charge on the metal (.. = −..)
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tion in the double layer. Such "maps of the double layer" can be given with reasonable certainty up to concentrations of about 1 N for mercury in contact with solutions of inorganic ions. However, this is-or was until very recently-the extent of the know­ ledge. The problems confronting a fundamental approach978-1-4684-1733-3978-1-4684-1731-9
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