| 书目名称 | Catalysis with Supported Size-selected Pt Clusters |
| 副标题 | Fundamental UHV and |
| 编辑 | Florian Frank Schweinberger |
| 视频video | http://file.papertrans.cn/223/222470/222470.mp4 |
| 概述 | Nominated as an outstanding Ph.D. thesis by the Technische Universität München, Germany.Shows new size-dependent reactions under UHV conditions on clusters and compares them to single-crystal data in |
| 丛书名称 | Springer Theses |
| 图书封面 |  |
| 描述 | In his thesis, Florian Schweinberger investigates the influence of the precise size of catalytically active species on reactivity. In order to do this he carries out studies both in UHV and under ambient conditions for supported, size-selected Platium clusters (8-68 atoms). Schweinberger probed the electronic structure, adsorption properties and reactivity of two olefins on surfaces and Pt clusters in the submonolayer range. With adsorbed trichloroethene (TCE) a possible cluster-adsorbate induced change in the electronic structure, and for ethene a low-temperature, size-dependent self-/hydrogenation was observed.In a collaborative approach, Schweinberger and colleagues investigated Pt clusters under ambient pressure conditions. They characterised the clusters at at the local and integral level and tested for temperature stability. Experiments in gas phase ?-reactors and in liquid, as part of a hybrid photocatalytic system, revealed size-dependent reactivity.Overall this thesis is not only of interest for those who want to perform similar experiments but also provides superb scientific insights for researchers in the field. |
| 出版日期 | Book 2014 |
| 关键词 | Applied Ambient Model Catalyst Experiments; CO Oxidation; Ethylene Hydrogenation; Laser Evaporation Clu |
| 版次 | 1 |
| doi | https://doi.org/10.1007/978-3-319-01499-9 |
| isbn_softcover | 978-3-319-37814-5 |
| isbn_ebook | 978-3-319-01499-9Series ISSN 2190-5053 Series E-ISSN 2190-5061 |
| issn_series | 2190-5053 |
| copyright | Springer International Publishing Switzerland 2014 |
|Archiver|手机版|小黑屋|
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