Titlebook: C-H Bond Activation and Catalytic Functionalization I; Pierre H. Dixneuf,Henri Doucet Book 2016 Springer International Publishing Switzerl

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书目名称C-H Bond Activation and Catalytic Functionalization I读者反馈学科排名

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,Rh(III)- and Ir(III)-Catalyzed Direct C–H Bond Transformations to Carbon–Heteroatom Bonds,II) and Ir(III) complexes played an important role to understand the nature of C.H bond activation. While numerous stoichiometric reactions of hydrocarbons with Rh(III) or Ir(III) complexes were scrutinized, their use in catalytic transformations has been relatively undeveloped until recently. Given

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,New Arylating Agents in Pd-Catalyzed C–H Bond Functionalization of 5-Membered Ring Heteroarenes,–carbon bonds. In most cases, aryl halides were employed as the coupling partners. However, since a few years, several new coupling partners have emerged as useful alternatives for such couplings. This chapter focuses on the recent advances on the discovery of new arylating agents in the palladium-c

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,Functionalization of [60]Fullerene via Palladium-Catalyzed C–H Bond Activation,terocycles and carbocycles have been obtained. The synthesis of [60]fullerene-fused indolines, isoquinolinones, azepines, tetrahydroisoquinolines, tetrahydrobenzazepines, sultones, tetrahydrobenzooxepines/isochromans, and dihydrophenanthrenes has been achieved by the palladium-catalyzed reactions of

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,Ruthenium(II)-Catalysed Functionalisation of C–H Bonds with Alkenes: Alkenylation versus Alkylation, heterocycles, alkenes and ferrocene derivatives on their reaction with alkenes, either via oxidative dehydrogenation to produce functional alkenes or via formal insertion of alkene into C–H bonds to afford alkylated products. The regioselectivity of . C–H bond alkenylation or alkylation is shown t

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,Ruthenium-Catalyzed C−N and C−O Bond-Forming Processes from C−H Bond Functionalization,ynthetic methods for the construction of C−N and C−O bonds through the activation of inert sp. and sp. C−H bonds is enumerated. The effect of a directing group (DG) for the chemo- and regioselective introduction of heteroatoms in the molecule replacing the unactivated C−H bonds is discussed.

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,,- and ,-Selective C–H Functionalization by C–H Activation,n addition to various strategies for .-selective functionalization via chelation assistance, organometallic C–H activation has recently enabled novel functionalizations of (hetero)arenes at remote .- or .-positions. The .- and .-selectivity was governed either by the inherent substrate structure or

Anhydrous

,Ruthenium-Catalyzed C−N and C−O Bond-Forming Processes from C−H Bond Functionalization,ynthetic methods for the construction of C−N and C−O bonds through the activation of inert sp. and sp. C−H bonds is enumerated. The effect of a directing group (DG) for the chemo- and regioselective introduction of heteroatoms in the molecule replacing the unactivated C−H bonds is discussed.