| 书目名称 | XUV Pump-Probe Experiments on Diatomic Molecules |
| 副标题 | Tracing the Dynamics |
| 编辑 | Kirsten Schnorr |
| 视频video | |
| 概述 | Nominated as an outstanding Ph.D. thesis by Max Planck Institute for Nuclear Physics, Heidelberg, Germany.Introductory chapters with numerous clear illustrations make the topic accessible to non-exper |
| 丛书名称 | Springer Theses |
| 图书封面 |  |
| 描述 | This book explores the relaxation dynamics of inner-valence-ionized diatomic molecules on the basis of extreme-ultraviolet pump-probe experiments performed at the free-electron laser (FEL) in Hamburg. Firstly, the electron rearrangement dynamics in dissociating multiply charged iodine molecules is studied in an experiment that made it possible to access charge transfer in a thus far unexplored quasimolecular regime relevant for plasma and chemistry applications of the FEL. Secondly the lifetime of an efficient non-radiative relaxation process that occurs in weakly bound systems is measured directly for the first time in a neon dimer (Ne.2.). Interatomic Coulombic decay (ICD) has been identified as the dominant decay mechanism in inner-valence-ionized or excited van-der-Waals and hydrogen bonded systems, the latter being ubiquitous in all biomolecules. The role of ICD in DNA damage thus demands further investigation, e.g. with regard to applications like radiation therapy. |
| 出版日期 | Book 2015 |
| 关键词 | Efficient Non-radiative Relaxation Process; Electron Rearrangment Dynamics; Excited van-der-Waals and |
| 版次 | 1 |
| doi | https://doi.org/10.1007/978-3-319-12139-0 |
| isbn_softcover | 978-3-319-36555-8 |
| isbn_ebook | 978-3-319-12139-0Series ISSN 2190-5053 Series E-ISSN 2190-5061 |
| issn_series | 2190-5053 |
| copyright | Springer International Publishing Switzerland 2015 |
发表于 2025-3-21 19:48:32
